Superconducting pairing and the pseudogap in the nematic dynamical stripe phase of La2−xSrxCuO4

Abstract

Fully absorption coefficient corrected Raman spectra were obtained in La2−xSrxCuO4. The B1g spectra have a Fleury–Loudon type two-magnon peak (resonant term) whose energy decreases from 3180 cm−1 (394 meV) to 440 cm−1 (55 meV) on increasing the carrier density from x = 0 to 0.25, while the B2g spectra have a 1000–3500 cm−1 (124–434 meV) hump (hill) whose lower-edge energy increases from x = 0 to 0.115 and then stays constant to x = 0.25. The B2g hump is assigned to the electronic scattering (non-resonant term) of the spectral function with magnetic self-energy. The completely different carrier density dependence arises from anisotropic magnetic excitations of spin–charge stripes. The B1g spectra were assigned to the sum of k ∥ and k⊥ stripe excitations and the B2g spectra to k⊥ stripe excitations according to the calculation by Seibold and Lorenzana (2006 Phys. Rev. B 73 144515). The k ∥ and k⊥ stripe excitations in fluctuating spin–charge stripes were separately detected for the first time. The appearance of only k⊥ stripe excitations in the electronic scattering arises from the charge hopping perpendicular to the stripe. This is the same direction as the Burgers vector of the edge dislocation in metal. The successive charge hopping in the Burgers vector direction across the charge stripes may cause Cooper pairs as predicted by Zaanen et al (2004 Ann. Phys. 310 181). Indeed, this is supported by the experimental fact that the superconducting coherent length coincides with the inter-charge stripe distance in the wide carrier density range. The one-directional charge hopping perpendicular to the stripe causes the flat Fermi surface and the pseudogap near (π,0) and (0,π), but the states around (π/2,π/2) cannot be produced. The low-energy Raman scattering disclosed that the electronic states at the Fermi arc around (π/2,π/2) are coupled to the A1g soft phonon of the tetragonal–orthorhombic phase transition. This suggests that the Fermi arc is produced by the electron–phonon interaction. All the present Raman data suggest that Cooper pairs are formed at moving edge dislocations of dynamical charge stripes.