Abstract

The behavior of Fano resonance and the reversal of near field optical binding force of dimers over different substrates have not been studied so far. Notably, for particle clustering and aggregation, controlling the near filed binding force can be a key factor. In this work, we observe that if the closely located plasmonic cube homodimers over glass or high permittivity dielectric substrate are illuminated with plane wave, no reversal of lateral optical binding force occurs. But if we apply the same set-up over a plasmonic substrate, stable Fano resonance occurs along with the reversal of near field lateral binding force. It is observed that during such Fano resonance, stronger coupling occurs between the dimers and plasmonic substrate along with the strong enhancement of the substrate current. Such binding force reversals of plasmonic cube dimers have been explained based on the observed unusual behavior of optical Lorentz force during the induced stronger Fano resonance and the dipole-dipole resonance. Although previously reported reversals of near field optical binding forces were highly sensitive to particle size/shape (i.e. for heterodimers) and inter-particle distance, our configuration provides much relaxation of those parameters and hence could be verified experimentally with simpler experimental set-ups.

Highlights

  • For particle clustering, particle aggregation and for improved sensors, controlling the near filed binding force is considered as a key factor

  • We have demonstrated that from the interplay between localized surface plasmon and propagating surface plasmon polariton along with the strong coupling between the two particles with the plasmonic substrate, the reversal of the optical binding force occurs during the strong Fano resonance

  • It should be noted that the binding force at DD resonance mode behaves quite differently for these two cases: (i) Far from the substrate- strong mutual attractive force occurs and (ii) very close [i.e. 5 nm away from spacer as shown in Fig. 2 (j)–(l)] to the substrate- strong mutual repulsive force occurs [the reversal mainly occurs before this dipole resonance at the strong Fano resonance, when stronger coupling with the plasmonic substrate starts to occur]

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Summary

Introduction

For particle clustering, particle aggregation and for improved sensors, controlling the near filed binding force is considered as a key factor. Still no investigation has been carried out regarding the behavior of both Fano resonance and the reversal of near field optical binding force with respect to the inter particle distance of two dimers over different substrates.

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