Abstract
Accurate values of the parallel and perpendicular components of g-factor and hyperfine coupling tensor were determined for [CrOCln]—(n−3) where n=4 and 5, by the ESR line shape analysis. It was shown by a molecular orbital treatment that these magnetic parameters can be explained consistently by taking into account of an excited electronic configuration in which an electron in a filled orbital is excited to the half-filled level. An assignment of a hitherto unexplained visible absorption band was proposed on the same ground.
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