Abstract
The pollutants from the marine exhaust gas seriously threaten air quality and human health. Wet absorption is one of the most efficient NOx control pathways. The strict emission control regulations require the wet NOx control technology to have high NOx removal efficiency and the nitrate concentration of the absorption solution to be below 60 mg/L. The novel system of ozone-Na2SO3/(NH2)2CO could not only make the NOx absorption efficiency and the amount of nitrate residue fully meet the regulations but also effectively reduce the (NH2)2CO consumption and the nitrite concentration. The final product of NO was mainly N2 instead of nitrate. The effects of O3 concentration, Na2SO3 concentration, (NH2)2CO concentration, O2 concentration, SO2 concentration, initial pH value, and temperature were thoroughly investigated. The experimental results showed that the NOx removal efficiency was mostly influenced by the O3 concentration, Na2SO3 concentration, and the initial pH value. Moreover, the nitrate concentration was mainly controlled by Na2SO3 concentration and initial pH value. While the nitrite concentration was governed by the (NH2)2CO concentration and initial pH value. The increase of O3 concentration and Na2SO3 concentration promote NOx absorption. Although the decrease of initial pH value resulted in a slight increase of nitrate, it greatly reduced the content of nitrite. Furthermore, the increase of Na2SO3 concentration helped to improve the NOx removal efficiency and inhibited the generation of nitrate. Initial pH value was the critical parameter for the NO absorption process. Ozone-Na2SO3/(NH2)2CO composite system showed great application potential in the field of marine wet NOx control technology.
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