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Abstract
Comparative study of the molecular dynamics of two xanthene dye derivatives (Rhodamine-6G and Fluorescein-548) is reported using spectrally resolved three-pulse photon echo spectroscopy. An appreciable change in the coherence and population dynamics was observed between the two xanthene derivatives due to the presence of different functional groups. Solution of Rhodamine-6G in methanol behaves in a more coherent fashion compared to that of Fluorescein-548 dye.
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