Abstract

Zero-field-cooled and field-cooled magnetization data in single-crystalline Nd0.5Sr0.5MnO3 revealed the existence of thermodynamic irreversibility below Curie temperature (TC), indicating the presence of frustration of spins. The imaginary part of ac susceptibility (χ″) indicates a prominent cusp below TC, which shifts to higher temperatures with increasing frequency. Magnetization, ac susceptibility, resistivity, and specific-heat measurements were used to find three critical exponents α=0.12(1), β=0.5(0), and γ=1.02(2). The values of the critical exponents are all between mean-field values and three-dimensional Heisenberg model values.

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