Abstract

In the frame of EUROMET Project No 325 “Analysis of Plutonium Alpha-Particle Spectra”, the isotopic composition of a 238,239,240Pu mixture was measured by mass spectrometry and by high-resolution alpha-particle spectrometry. The latter revealed a discrepancy with published data of the alpha-particle emission probabilities ( P α ) and the energies ( E α ) of the two major peaks of 240Pu. New values have been derived: P α1 =0.7256 (6), P α2 =0.2735 (7) and E α1 =5168.54 (14) keV, E α2 =5124.10(15) keV, relative to reference peaks of 238Pu and 239Pu.

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