Abstract
A new strategy for the preparation of molecular magnets by the reduction of phthalocyanines with strong metallocene donors has been suggested. Compound (Cp*2Cr+)·(FeIPc−)·(C6H4Cl2)4 (1) contains uniform stacks of alternating closely packed Cp*2Cr+ and FeIPc− ions. 1 is a soft ferrimagnet showing hysteresis with a small coercive field and a bifurcation temperature of about 5 K.
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