Abstract
Pellet porosity and specific surface area variations caused both by sintering and chemical reaction have been determined for the manganese oxide-manganese sulfide system. Sintering data for the pure solids have been correlated as a function of time and temperature; property variations due to reaction were determined at low temperature where sintering was unimportant. The separate correlations have been combined in a manner such that reasonable predictions of properties in a mixed oxide-sulfide system subject to simultaneous reaction and sintering are possible. All parameter correlations are in a form suitable for inclusion in an appropriate gas-solid reaction model. While the numerical results are specific to the system studied, the methodology should be generally applicable to gas-solid reaction systems where property variations must be considered.
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