Abstract

In condensed-phase molecular systems, and particularly insulating molecular crystals, infrared and Raman spectroscopies are well-established tools for investigating molecular and crystalline structural properties.1 On the other hand, in inorganic semiconductors and metals the same spectroscopic methods are widely used to evaluate electronic band structure parameters.2 Organic charge transfer (CT) crystals, as molecular conductors and semiconductors, share some properties of both the above classes of solids, and, therefore, new spectroscopic phenomena are expected, and indeed observed for these materials.3 KeywordsOscillator StrengthCharge Transfer TransitionDimeric ModelMolecular ConductorResonance Raman ScatteringThese keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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