Abstract
Enhancing the activity of oxygen evolution reaction (OER) is crucial for improving the efficiency of electrochemical water splitting (EWS). The highly adjustable electronic structure and potential high conductivity of transition metal sulfides (TMSs) make them promising candidates for OER electrocatalysts. Herein, we have synthesized trimetallic sulfides Fe2Ni1Zn1–S(II) based on layered double hydroxides (LDHs) precursor employing a facile and efficient two-step solvothermal approach. Benefitting from the multi-metallic synergistic effect and the distinctive interfacial structure, Fe2Ni1Zn1–S(II) shows excellent electrocatalytic OER performance (η10 = 252 mV, Tafel slope = 64.2 mV∙dec−1). Meanwhile, it has outstanding stability (50 h) in 1 M KOH, which is better than RuO2 and many other metal sulfide electrocatalysts. Furthermore, it was found that the structure of the catalyst was still retained after OER test, which further verified its catalytic stability. This work supplies an effective route for the preparation of LDHs derived multi-metallic sulfides.
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