Abstract
The quadrupole resonance spectra and the quadrupole spin-lattice relaxation times of the35Cl nuclei are correlated with the molecular structures of the two chlorine-containing diazadienes CCl3CCl=NCCl=NC6H5 and CCl3CCl=NCCl=NCCl2CCl3. The monotropic polymorphism found in the case of the second crystal is discussed.
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