Strong terahertz matter interaction induced ultrasensitive sensing in Fano cavity based stacked metamaterials

Abstract

Strong interaction between terahertz (THz) and matter is a topic of paramount importance, considering continuously enhanced interest in THz photonics as well as condensed matter physics, which can lead to the observation of many linear and nonlinear phenomena in the THz regime. Here, we demonstrate a unique and novel metamaterial-based technique of strong THz matter interaction towards thin film sensing, where the analyte is sensed in between the stacked metasurfaces forming the Fano cavity. Sub-wavelength structures typically overcome the diffraction limit of any optical system, which also possess very high confinement of electromagnetic energy. Fano resonance possesses a sharp asymmetric line shape, low radiation loss and large tuning capability. In addition to them, the material under test is placed in between the metasurfaces to utilize the substantial energy confinement leading to strong light matter interaction, a scheme never explored before. By intelligently exploiting the above characteristics, we have demonstrated a novel way to detect both the refractive index (dielectric constant), thickness and loss factor of the material under test when placed between the array of the meta-resonators forming the Fano metamaterials. Our study revealed that the sensitivity and figure of merit (FOM) are strikingly different for dipole and Fano modes. A maximum sensitivity of >1 THz RIU−1 (1.76 × 105 nm RIU−1) and FOM of around 14.05 are achieved at the Fano mode. Additionally, our sensor shows better performance with decreasing spacer thickness (lesser the material, more the sensitivity). Moreover, the proposed device is passive towards typical ambience temperature variation, and is highly compact because of its stacked configuration. The demonstrated device can be extremely beneficial towards realizing ultra-sensitive meta-sensors and other miniaturized THz meta-photonic devices, and bio-chemical sensing where strong light matter interaction is mandatory.