Abstract

We report on semi-transparent stretchable Ag films coated on a wavy-patterned polydimethylsiloxane (PDMS) substrate for use as stretchable electrodes for stretchable and transparent electronics. To improve the mechanical stretchability of the Ag films, we optimized the wavy-pattern of the PDMS substrate as a function of UV-ozone treatment time and pre-strain of the PDMS substrate. In addition, we investigated the effect of the Ag thickness on the mechanical stretchability of the Ag electrode formed on the wavy-patterned PDMS substrate. The semi-transparent Ag films formed on the wavy-patterned PDMS substrate showed better stretchability (strain 20%) than the Ag films formed on a flat PDMS substrate because the wavy pattern effectively relieved strain. In addition, the optical transmittance of the Ag electrode on the wavy-patterned PDMS substrate was tunable based on the degree of stretching for the PDMS substrate. In particular, it was found that the wavy-patterned PDMS with a smooth buckling was beneficial for a precise patterning of Ag interconnectors. Furthermore, we demonstrated the feasibility of semi-transparent Ag films on wavy-patterned PDMS as stretchable electrodes for the stretchable electronics based on bending tests, hysteresis tests, and dynamic fatigue tests.

Highlights

  • Ag wrinkled electrodes on the oxygen plasma and Sodium Dodecyl treated PDMS substrates as a metal electrode for wearable wireless sensor[27]

  • We compared the mechanical properties of thin Ag electrodes sputtered on flat PDMS and wavy-patterned PDMS substrates, and we suggest that thin Ag films on wavy-patterned PDMS are feasible for stretchable electrodes

  • Cross-links on the surface region of the PDMS substrate are significantly affected by UV ozone (UVO) irradiation time

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Summary

Introduction

Ag wrinkled electrodes on the oxygen plasma and Sodium Dodecyl treated PDMS substrates as a metal electrode for wearable wireless sensor[27]. Wrinkled or wavy-patterning methods for PDMS substrates have been previously reported, there have been no reports on the electrical, optical, and mechanical properties of very thin Ag films coated on wavy-patterned PDMS substrates as stretchable and semi-transparent electrodes for stretchable and transparent interconnectors or stretchable and transparent thin film heaters. We reports on the characteristics of thin Ag films coated on wavy-patterned PDMS substrates to use as stretchable electrodes. We compared the mechanical properties of thin Ag electrodes sputtered on flat PDMS and wavy-patterned PDMS substrates, and we suggest that thin Ag films on wavy-patterned PDMS are feasible for stretchable electrodes. For a precise pattern of the semi-transparent Ag interconnectors, the wavelength and amplitude of the wavy-pattern of PDMS substrate were controlled by the extent of pre-strain and UV-ozone treatment time. We demonstrated the outstanding stretchability of semi-transparent Ag films in two applications: stretchable and semi-transparent interconnectors and semi-transparent electrodes for stretchable and transparent thin film heaters

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