Abstract

Topological insulators are potentially transformative quantum solids with metallic surface states which have Dirac band structure and are immune to disorder. Ubiquitous charged bulk defects, however, pull the Fermi energy into the bulk bands, denying access to surface charge transport. Here we demonstrate that irradiation with swift (∼2.5 MeV energy) electron beams allows to compensate these defects, bring the Fermi level back into the bulk gap and reach the charge neutrality point (CNP). Controlling the beam fluence, we tune bulk conductivity from p- (hole-like) to n-type (electron-like), crossing the Dirac point and back, while preserving the Dirac energy dispersion. The CNP conductance has a two-dimensional character on the order of ten conductance quanta and reveals, both in Bi2Te3 and Bi2Se3, the presence of only two quantum channels corresponding to two topological surfaces. The intrinsic quantum transport of the topological states is accessible disregarding the bulk size.

Highlights

  • Topological insulators are potentially transformative quantum solids with metallic surface states which have Dirac band structure and are immune to disorder

  • Three-dimensional (3D) topological insulators are a spectacular example of this1—narrow-band semiconductors, well known for their high performance as thermoelectrics[2], they were discovered to support unusual gapless robust two-dimensional (2D) surface states that are fully spin-polarized with Dirac-type linear electronic energy-momentum dispersion[3,4], which makes them protected against backscattering by disorder[3,4,5,6]

  • We demonstrate that bulk conductivity in topological insulators (TIs) can be decreased by orders of magnitude to charge neutrality point on a large scale by the controlled use of electron beams, which for energies below B3 MeV are known to produce a well-defined, stable and uniform spread of Frenkel pairs[15] within their penetration range of hundreds of micrometres

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Summary

Introduction

Topological insulators are potentially transformative quantum solids with metallic surface states which have Dirac band structure and are immune to disorder. We demonstrate that bulk conductivity in topological insulators (TIs) can be decreased by orders of magnitude to charge neutrality point on a large (depth) scale by the controlled use of electron beams, which for energies below B3 MeV are known to produce a well-defined, stable and uniform spread of Frenkel (vacancy-interstitial) pairs[15] within their penetration range of hundreds of micrometres.

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