Abstract
Thermochemical values, ΔH0n−1,n and ΔS0n−1,n, for clustering reactions, Rg+n−1+2Rg=Rg+n+Rg (Rg=He, Ne, Kr, and Xe), were measured with a pulsed electron-beam mass spectrometer. The −ΔH0n−1,n values show a sudden decrease between n=3 and 4, for all rare gases suggesting that the core ion in Rg+n is Rg+3. The values −ΔH0n−1,n with n=3 are found to be in the order Ne<He<Ar<Kr<Xe, and those with n≥4 in the order of atomic radii.
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