Abstract

We discuss the stability of ferromagnetic long-range order in three-dimensional classical XY ferromagnets upon substitution of a small subset of equally oriented bonds by impurity bonds, on which the ferromagnetic exchange J_perp > 0 is replaced by a strong antiferromagnetic coupling J_imp < 0. In the presence of a single impurity bond, once the absolute value of the frustrating coupling J_imp < 0 exceeds a threshold J_c > 0, the ground state becomes two-fold degenerate, corresponding to either clockwise or anticlockwise canting of the spins in the vicinity of the impurity bond. In the presence of a small concentration of impurity bonds, the effective low-energy Hamiltonian is that of Ising variables encoding the sense of rotation of the local canting around the impurities. Those degrees of freedom interact through a dipolar interaction mediated by spin waves. A ferromagnetic Ising ground state indicates the instability of the XY ferromagnet towards a spiral state with a wave vector proportional to the concentration of impurity bonds. To analyze under which circumstances such a ground state arises, we study first impurities forming superlattices. For a subclass of those, we can rigorously establish the existence of spiral order. For another class of superlattices, the Ising variables order ferromagnetically in planes perpendicular to the orientation of impurity bonds, but antiferromagnetically parallel to it, which results in a fan-like XY ground state. Second, we consider the case when the impurity bonds are randomly distributed on the three-dimensional host lattice according to a Poisson process. We show the phenomenon of spiral order by disorder with an ordering wave vector proportional to the impurity concentration. The analytical predictions are confirmed by Monte Carlo simulations and are relevant for magnetic materials such as YBaCuFeO_5.

Highlights

  • Insulating magnets supporting long-range magnetic spiral order are of technological interest as they can display magnetically induced ferroelectricity [1,2,3,4]

  • In order to engineer magnetic insulators with magnetic spiral order established at high temperatures, it is of fundamental interest to investigate analogous mechanisms

  • The spin wave encoded by the angle θr is the gapless Goldstone mode associated with the spontaneous breaking of the O(2) spin symmetry by the ferromagnetic ground state

Read more

Summary

INTRODUCTION

Insulating magnets supporting long-range magnetic spiral order are of technological interest as they can display magnetically induced ferroelectricity [1,2,3,4]. A single impurity bond does not destroy the ferromagnetic long-range order of the ground state It does result in a canting of the classical XY spins in the vicinity of the impurity bond, provided the local frustration is sufficiently strong, i.e., |Jimp| Jc for some threshold value Jc > 0. Its solution is compared to Monte Carlo simulations of a model with the same network of exchange interactions, but in which the classical XY spins are replaced by classical Heisenberg spins with an additional easy-plane anisotropy The latter allows for close contact with experimentally realized magnets, such as YBaCuFeO5 and layered perovskites, which are believed to embody the physical ingredients and mechanisms discussed above.

Definition of the XY model
Impurity-free case
Periodic boundary conditions
Case of a dilute set of impurity bonds
Boundary conditions along the z axis
SUPERLATTICES OF IMPURITY BONDS
Analytical considerations
Comparison between analytical and numerical results for superlattices
Spiral phase in a realistic model for YBaCuFeO5
Dependence of the ground state on the superlattice of impurity bonds
Limit of dilute impurities
Cubic superlattices
RANDOM IMPURITIES
FINITE-TEMPERATURE TRANSITION TO THE SPIRAL PHASE
Mean-field theory
Dipolar approximation
Comparison to simulations in the XY model and to experiments
CONCLUSION AND OUTLOOK
Full Text
Published version (Free)

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call