Abstract

The specific heat, the susceptibility under pressure, and the dielectric constant were measured for single crystals ${\mathrm{Y}}_{1\ensuremath{-}x}{\mathrm{La}}_{x}{\mathrm{TiO}}_{3}$. The observed ${T}^{2}$-dependent specific heat at low temperatures for $0.17\ensuremath{\le}x\ensuremath{\le}0.3$ samples shows a spin-orbital liquid state between the ferromagnetic/orbital ordering $(xl0.17)$ and antiferromagnetic/possible orbital liquid phase $(xg0.3)$. The nonmonotonous pressure dependence of ${T}_{\text{C}}$ and the glassy behavior of the dielectric loss for the $x=0.23$ sample suggest that it is approaching a possible quantum critical point. All these properties result from the coupling between the strong spin and orbital fluctuations while approaching the phase boundary.

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