Abstract
Abstract An anomaly reported in the spin-lattice relaxation of Co 2+ in (NH 4 ) 2 (Co, Zn)(SO 4 ) 2 6H 2 O is explained in terms of cross-relaxation to faster-relaxing Ni 2+ impurities. The explanation is supported by measurements on crystals with and without Ni added; in the absence of Ni no anomaly is observed, and the relaxation of the Co is attributable to the usual Van Vleck process.
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