Abstract
AbstractThe isotropic and anisotropic ESR spectra of dialkyl oxalate radical anions, including derivatives which were labelled with 13C or 17O in the carbonyl and 2H or 13C in the alkyl groups, were measured. The spin density distribution as determined from the experimental nuclear hyperfine coupling constants agrees very well with MNDO‐CI calculations. As a consequence of the strictly planar structure of the radical anions, E/Z isomers are observed.
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