Abstract
AbstractThe wide spectral range of the solar flux with undesirable diffused energy distribution remains a substantial impediment to the high‐efficiency utilization of the whole spectrum. Here, inspired by the spectrally selective sunlight utilization of plants, a spectrum‐tailored solar harnessing aerogel is conceived. It is composed of oxygen vacancy (Ov) defect‐rich semiconductor HNb3O8 (D‐HNb3O8) nanosheets and polyacrylamide (PAM) framework to perform all‐in‐one photochemical and photothermal full solar energy conversion. The aerogel selectively utilizes the whole solar spectrum, in which high energy ultraviolet (UV) photon is converted into high redox potential electron–hole pairs, while low energy visible‐near infrared (NIR) photons are transformed into heat. The designed solar absorber‐polymer composite shows energy harnessing‐conversion capability with desired heat insulation, reactant enrichment, rapid mass diffusion and capillary pumping characteristics, thus realizing a high efficient steam generation and photochemical activity. This cooperative photochemical and photothermal solar energy conversion, at respective optimal working spectrum, holds great promise for optimizing and maximizing the solar energy utilization, as well as opening up opportunities to explore simultaneous multifunctional usage of solar energy.
Sign-in/Register to access full text options 
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
