Abstract
The theory of third harmonic generation of MX complex is presented on the basis of charge density wave model. The recently observed spectrum χ(3) (ω) of Pt-Cl complex can be well interpreted by this theory, which shows that the experimental peak at 1.8eV is produced by the two-photon resonance between the bottom of valence band and the top of conduction band. Besides, our theory predicts that there exist another peak below the observed region.
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