Abstract
A consistent quantum approach to calculating the electron–nuclear γ transition spectra (a set of vibration–rotational satellites in a molecule) of a nucleus in the multiatomic molecules is proposed and generalizes the well-known Letokhov–Minogin model. Estimates of the vibration–nuclear transition probabilities in a case of the emission and absorption spectrum of nucleus 188Os in the molecule of OsO4 and nucleus 191Ir in the molecule IrO4 are presented.
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