Abstract
Abstract : During the last grant period, we have used negative ion photoelectron spectroscopy (PES) and ZEKE spectroscopy to probe the spectroscopy and dynamics of negatively-charged and neutral species. Specific areas include (a) ZEKE spectroscopy of diatomic rare gas halides RgX(-)and clusters of the form Rg(n)X(-), (b) PES of I2(-)Ar(n) and I2(-) (CO2)n, in which the effects of solvation on a molecular (as opposed to atomic) ion are probed, (c) PES as a probe of neutral radicals and reactive intermediates, specifically I(3), CH3O, and NCN, and (d) time-resolved studies of excited state dynamics in I(-)(H2O)(n) clusters using femtosecond photoelectron spectroscopy (FPES).
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