Abstract
Theoretical prediction is made for various types of molecular Zeeman spectroscopy due to a circularly polarised pump laser, in which optical rectification produces a pattern of spectral splitting mediated by the imaginary antisymmetric part of the frequency-dependent molecular polarisability. The hyperfine part of this splitting, in which the nuclear spin quantum number plays a role, leads to the expectation of laser-induced resonance effects akin to conventional nuclear magnetic resonance (NMR) and electron spin resonance (ESR). Experimental conditions for the observation of "laser Zeeman" spectral effects are defined using double resonance and saturation in mode-locked lasers for ultra high resolution.
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