Abstract

Surface fine particulate matter (PM) with a diameter of less than 2.5 microns (PM2.5) negatively impacts human health and the economy. However, due to data and model limitations, obtaining high-quality, high-spatial-resolution surface PM2.5 concentration data is a challenging task, and it is difficult to accurately assess the temporal and spatial changes in PM2.5 levels at a small regional scale. Here, we combined multi-angle implementation of atmospheric correction (MAIAC) aerosol products, ERA5 reanalysis data, etc., to construct an STW-LightGBM model that considers the spatiotemporal characteristics of air pollution and estimate the PM2.5 concentration of China’s surface at 1 km resolution from 2015 to 2020. Our model performed well, and the fitting accuracy of the 10-fold cross-validation between years was 0.877–0.917. The fitting accuracy of the model was >0.85 at different time scales (month, season, and year). The average slope of the regression prediction was 0.9 annually. The results showed that PM2.5 pollution improved from 2015 to 2020. The average PM2.5 concentration decreased by 4.55 μg/m3, and the maximum decrease reached 90.51 μg/m3. The areas with high PM2.5 concentrations were predominantly in the North China Plain, Sichuan Basin, and Xinjiang in the west, and the levels in areas with elevated PM2.5 levels were consistent across most study years. The standard deviation ellipse for PM2.5 in China showed a ‘northeast–southwest’ spatial distribution. From an interannual perspective, the average values of the four seasonal stations in the country showed a downward trend from 2015 to 2020, with the most obvious decline in winter, from 70.67 μg/m3 in 2015 to 46.75 μg/m3 in 2020. Compared to earlier inversion studies, this work provides a more stable and accurate method for obtaining high-resolution PM2.5 data, which is necessary for local air governance and environmental ecological construction at a fine scale.

Full Text
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