Spatiotemporal modulation of ultrafast plasmonic vortices with spin–orbit coupling

Abstract

The vortex field of surface plasmon polariton with orbital angular momentum (OAM), called plasmonic vortex, has played an important role in various research fields. However, the spatiotemporal properties of plasmonic vortex pulses excited by ultrafast laser, especially the dynamics of spin‒orbit coupling in the ultrafast plasmonic vortex field, have yet to be investigated deeply. Here, we study the spatiotemporal modulation of ultrafast plasmonic vortices with spin‒orbit coupling, using both analytical and simulation methods. The ultrafast plasmonic vortices are excited by a ring-shaped plasmonic lens, with an incident light composed of two time-delayed femtosecond sub-pulses carrying the same OAM but orthogonal circular polarizations. The dynamics of time-varying electric field, energy flow and angular momentum distributions of the plasmonic vortices are demonstrated, revealing details of the spin‒orbit coupling in spatiotemporal domain, such as the merging of multiple phase singularities with energy flow loops, and the variation of spin/orbital angular momentum per photon over time. This work could deepen the understanding of spin‒orbit coupling in plasmonic field and provide new ideas for ultrafast on-chip optical information processing.