Spatiotemporal coherence of mean and extreme aerosol particle events over eastern North America as observed from satellite

Abstract

Quantifying spatiotemporal scales of coherence and variability of aerosol particle properties provides (i) metrics for evaluating observational data sets and model simulations, (ii) inferences regarding dominant causes of variability, and (iii) information that is necessary to determine their climate forcing and air quality impacts. Accordingly, analyses of columnar aerosol optical depth (AOD) and Ångström exponent (AE) from the MODerate resolution Imaging Spectroradiometer (MODIS) on the Aqua and Terra satellites, and AErosol RObotic NETwork (AERONET) stations are used to evaluate the spatially averaged (Level-3) MODIS products, and to characterize the spatiotemporal scales of variability (and coherence) of aerosol particles over eastern North America (2000–2013). Results show a high degree of consistency in AOD retrievals from the different data sets but larger discrepancies in AE estimates, highest mean AOD and lowest day-to-day variability during the summer, and largest scales of spatial coherence in summer and fall. Consistent with the scales of spatial coherence from MODIS data, in both data sets power spectra indicate AOD variability is manifest primarily on synoptic and annual time scales. Conversely, AE variability in MODIS data is primarily focused on seasonal, semiannual, and annual time scales, and there is an additional mode of AE variability at ∼30 days in the AERONET measurements. The frequency of co-occurrence of extreme AOD values (>local 90th percentile) decreases to below 50% at ∼150 km from a central grid cell, but is above that expected by random chance over almost all of eastern North America, indicating supra-regional scale extreme events.