Abstract
HighlightsSolvation engineering toward dual-salt electrolyte by fluorosurfactant additive is proposed, which implements the stable interface of electrode/electrolyte coupled with fast ion thermodiffusion, improving the durability and capability of lithium-ion thermoelectrochemical cell.By combining the optimized electrolyte with functional electrodes, as-constructed device exhibits high Seebeck coefficient and energy density based on hybrid mechanisms, which can be extended as self-power supply for smart electronics.
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