Abstract

Does the title compound prefer OLi or CLi contacts in the solid state? OLi contacts are characteristic of lithiated phenylsulfones, CLi contacts of allyllithium compounds. According to the X-ray structure analysis, the chiral dimer 1 with OLi contacts is present in the crystal. The angle at C-1 corresponds to a middle position between sp3 and sp2 hybridization. These results also hold for the structure of 1 in solution.

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