Solar-pumped fiber laser with all-inorganic cesium lead halide perovskite quantum dots

Abstract

We demonstrate a low-concentrated solar-pumped fiber laser with all-inorganic cesium lead halide perovskite quantum dots (QDs), which function as a sensitizer. The perovskite QDs exhibit substantial advantages for solarpumped laser applications because of their broad absorption and narrow emission spectra with high quantum yield. We successfully tuned the peak emission wavelength of the perovskite QDs by altering the I/Br ratio in order to achieve spectral overlap with Nd3+ ions, which have been widely used as a laser medium for solar-pumped lasers. The measurement results show that the laser output power is highly sensitive to the peak emission wavelength of the QDs. Although our synthesized QDs have a quantum yield of approximately 65%, which is less than that of conventional organic dyes, the laser performance was comparable because the fluorescence spectrum is tailored to the Nd3+ absorption band.