Abstract

Heavy metal/ferromagnet interfaces feature emergent spin-orbit effects absent in the bulk materials. Because of their inherent strong coupling between spin, charge, and orbital degrees of freedom, such systems provide a platform for technologically sought-after spin-orbit torques (SOTs). However, the microscopic origin of purely interfacial antidamping SOT, especially in the ultimate atomically thin limit, has proven elusive. Here, using two-dimensional (2D) van der Waals materials as a test bed for interfacial phenomena, we address this problem by means of a microscopic framework accounting for band structure effects and impurity scattering on equal footing and nonperturbatively. A number of unconventional and measurable effects are predicted, the most remarkable of which is a giant enhancement of antidamping SOT in the dilute disorder limit induced by a robust skew scattering mechanism, which is operative in realistic interfaces and does not require magnetic impurities. The newly unveiled skew scattering mechanism activates rich semiclassical spin-charge conversion effects that have gone unnoticed in the literature, including a collinear Edelstein effect with nonequilibrium spin polarization aligned with the direction of the applied current.Received 14 May 2020Revised 19 August 2020Accepted 25 November 2020DOI:https://doi.org/10.1103/PhysRevResearch.2.043401Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasMagnetismMagnetoelectric effectRashba couplingSpin torqueSpin-orbit couplingSpintronicsPhysical Systems2-dimensional systemsBilayer filmsGrapheneTransition metal dichalcogenidesTechniquesBoltzmann theoryDiagrammatic methodsGreen's function methodsCondensed Matter, Materials & Applied Physics

Highlights

  • When a current is driven through a surface with broken inversion symmetry, a nonequilibrium spin polarization is induced due the spin-orbital-entangled character of electronic wave functions

  • Current-induced spin-orbit torques (SOTs) are conventionally classified into two broad categories depending on their behavior under time reversal T : the m-odd or fieldlike SOT that affects the precession around the effective magnetic field and the m-even or antidamping torque that renormalizes the Gilbert damping and is responsible for the magnetization switching [5,6,7]

  • We have reported a microscopic theory of SOT generated by 2D materials proximity coupled to a ferromagnet

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Summary

Introduction

When a current is driven through a surface with broken inversion symmetry, a nonequilibrium spin polarization is induced due the spin-orbital-entangled character of electronic wave functions. Current-induced spin-orbit torques (SOTs) are conventionally classified into two broad categories depending on their behavior under time reversal T : the m-odd or fieldlike SOT that affects the precession around the effective magnetic field and the m-even or antidamping torque that renormalizes the Gilbert damping and is responsible for the magnetization switching [5,6,7]. Fueled by the discovery of ferromagnetism in 2D materials, recent works have reported SOT switching of vdW-bonded ferromagnets (FMs), an important stepping stone toward the all-electrical control of atomically thin spin memories [8,9,10,11]. Experiments employing WTe2 [12,13,14], a transition

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