Abstract
An extension of our previous theory of spin relaxation by translational diffusion in two-dimensional (2D) systems is proposed by considering the very nonuniform radial molecular distribution observed at short intermolecular distance. This increases greatly the absolute values of the spin-lattice relaxation rates T−11 and enhances the size effects on their diffusion (or temperature) dependences. The existence of two maxima in these dependences should facilitate the interpretation of experimental data in 2D heterogeneous systems.
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