Abstract

ABSTRACTWe investigate nonequilibrium behavior of a polydisperse ensemble of fluid membrane vesicles by means of a diffusive Boltzmann transport equation which, incorporates vesicle diffusion and the reactions between vesicles. This approach is used to study the time evolution of the size distribution of an initially monodisperse vesicle ensemble and its interesting properties such as the internal aqueous, encapsulated volume. We investigate various nonequilibrium paths such ensembles may follow during the equilibration process.

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