Abstract
We study six-wave mixing (SWM) spectroscopy based on electromagnetically induced transparency in a Doppler-broadened cascade four-level system. It is found that the SWM spectra are extremely sensitive to the configuration of the incident beams, where the linewidth can be either Doppler-free or very broad, due to the polarization interference of atoms of different velocities. This polarization interference can be controlled in the presence of a strong coupling field. Moreover, SWM can be employed as a new type of Doppler-free Autler–Townes (AT) spectroscopy, which has better spectral resolution than conventional AT spectroscopy. Finally, we also reveal the intrinsic connection between frequency-domain SWM spectroscopy and time-domain photon echoes through studying the time-domain correspondence of SWM.
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