Single‐Scattering Properties of Encapsulated Fractal Black Carbon Particles Computed Using the Invariant Imbedding T‐Matrix Method and Deep Learning Approaches

Abstract

AbstractEfficient and accurate computation of the single‐scattering properties of black carbon (BC) aerosols is fundamental in various fields, including remote sensing and climate simulations. In this study, we developed a composite model of fractal aggregates of BC encapsulated with hygroscopic aerosols to represent the ambient BC. We used the invariant imbedding T‐matrix method to compute the optical properties of fully and partially encapsulated BC aerosols. In this new model, the traditional assumption of unoverlapped surfaces in the super‐position T‐matrix method is unnecessary. After extensive simulations, we established a database of single‐scattering properties, including the extinction efficiency, the single‐scattering albedo, the asymmetry factor and six phase matrix elements. Moreover, we obtained deep neural networks (DNNs) from this database using a deep learning method. These DNN models provide a universal interface for predicting the optical properties of ambient BC aerosols. Specifically, through a modified architecture of the DNN, we trained two models based on the database to predict three integrated optical properties (extinction efficiency, single‐scattering albedo, and asymmetry factor) and six phase matrix elements. We performed statistical assessments based on the true values in the database and the predicted values from the DNNs, demonstrating that the DNNs accurately predicted all single‐scattering properties. Therefore, the developed DNN models can be conveniently implemented in aerosol optical parameterization for remote sensing studies and atmospheric models.