Abstract
The cyanine distortion of doubly charged ethylenes leading to twisted molecular halves connected by a C–C single bond inciudes tetrakis(p-dimethylaminophenyl)ethylene, which on twofold oxidation with iodine increases its twist angle ω from 19 to 53° and its central CC bond length from 135 to 150 pm as predicted by PM3 calculations.
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