Abstract

A hexagonal CdSe crystal is excited with picosecond Nd:glass laser pulses. Two-photon absorption and resonant non-phasematched second harmonic generation occur simultaneously. Using different crystal orientations all components of the second harmonic susceptibility tensor and some components of the two-photon absorption susceptibility tensor are determined.KeywordsSecond Harmonic GenerationHarmonic GenerationPump PulseGlass LaserSusceptibility TensorThese keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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