Abstract
Abstract In the present study of the Rydberg spectra of the methyl and silyl radicals, with the molecule-adapted Quantum Defect Orbital (QDO) method, we have sought and found important analogies between the spectral intensities of analogous transitions in these isovalent molecules. Further similarities with the spectra of their isolated central atoms and their united atom limits has not only served the purpose of assessing the quality of our calculations, but may also offer some relevant practical use.
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