Abstract
Porous polymers are among the most promising porous materials for various application because they show the combined advantages of fluorescent porous materials and polymers. This study developed a cell imaging technique based on luminescent porous organosilicon polymers (LPOPs) that were synthesized via Friedel-Crafts reaction of octaphenylcyclotetrasiloxane with octavinylsilsesquioxanes. The porous organosilicon polymers possessed narrow pore-size distribution, high surface area, and monomodal nanopores centered at approximately 0.59 nm. The excellent properties to the porous polymers can be attributed to the fine structures of LPOPs. LPOP-2 owned the highest fluorescence intensity and micropore volume ratio in LPOPs and showed high selectivity for Fe3+ detection and excellent sensitivity to nitroaromatic compound detection. Interestingly, these porous polymers still exhibited excellent responsiveness to Fe3+ ion even when inside of living cells. We also fabricated a paper-based sensor using LPOP-2 to develop a simple method for visual detection of explosives. This rapid and visual paper sensor demonstrates promising application for explosive detection and can be expanded for the detection of other analytes.
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