Abstract
The supersonic beam method combined with techniques of laser spectroscopy has been applied to determine the repulsive wall of the D 10 +( 1Σ +) excited-state potential of CdAr and CdKr molecules. The molecules were produced in a continuous supersonic-expansion beam and excited with a dye-laser beam directly from the X 10 +( 1Σ +) to the excited state. Analysis of the laser-induced fluorescence of the unstructured continuum ← bound profiles, recorded for the first time in excitation at the D 10 + ← X 10 + transition, yielded information on the short range D 10 +-state potential of the molecules.
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