Abstract

Dense suspensions of non-Brownian particles may partially behave as thixotropic yield stress fluids. We study the flow of such fluids between two concentric cylinders using a phenomenological structural kinetics model. The structural kinetics approach balances the simplicity of phenomenological continuum approaches with a simplified model for structure against the complexity a more fundamental model based on particle micromechanics. A modified version of Houska’s model, which includes a diffusive term for the structural parameter, is considered. Depending on the breakdown rate of the structural parameter, shear-banding may be observed. For shear-banding in steady flows, the stress selection depends on the diffusion of the structural parameter. If there is no structural diffusion, the displacement of the interface between the flowing and the static regions fixes the stress at the interface during the transient flow. In the cases of very small diffusive coefficients, the stress at the fluid / solid interface converges to a limit value which is different from the yield stress of the structured material as expected without any diffusion. Nevertheless, the inner torque and the flow profile are quite similar in both cases and the differences are localized near the fluid / solid interface. For shear-banding, the gradients of the structural parameter and the strain rate are very abrupt but the continuity is preserved by the diffusion.

Highlights

  • Dense suspensions of non-Brownian particles exhibit a very rich behavior such as yield stress and shear-banding [1, 2] that remain incompletely understood

  • We focus on the shear banding in localized flows

  • The diffusive term of the structural parameter selects the stress in case of shear-banded flows

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Summary

Introduction

Dense suspensions of non-Brownian particles exhibit a very rich behavior such as yield stress and shear-banding [1, 2] that remain incompletely understood. Shear-banding has been studied in visco-elastic context [3, 4] but recent work [5] exhibits a different mechanism for shear-banding predicted by a visco-plastic thixotropic model. Fardin et al [7] show that the length based on this stress diffusion is at the order of magnitude of the molecular size in worm-like micelles. For non-Brownian suspensions, the velocity profiles obtained by Fall et al [2] suggests that the diffusion length is at the order of magnitude of the particle size, if such diffusive mechanism plays a role in the flow. The existence of a critical shear rate γc in thixotropic yield stress fluids is often explained in terms of an underlying decreasing branch of the flow curve at low shear rates [8]. Results obtained with and without structural diffusion are compared, especially when the diffusion coefficient is evanescent

Modified Houska’s model
Boundary conditions for the flow
Numerical method
Diffusive stress selection
Transient flows
Start unyielded
Conclusion
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