Abstract
The gas-liquid isotopic exchange between BF3 and the n-butyl sulfide-BF3 complex was studied as a possible system for enriching boron isotopes. The single stage separation factor varied from 1.054 at —20°C to 1.033 at 26°C. B10 concentrated in the liquid phase. The heat of association of the n-butyl sulfide-boron trifluoride complex was determined to be —12.76±0.06 kcal/mole from a series of vapor pressure measurements of the complex made at several mole ratios of BF3 to sulfide.
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