Abstract

Abstract. Atmospheric transport of traces gases and aerosols plays an important role in the distribution of air pollutants and radiatively active compounds. For model simulations of chemistry-climate interactions it is important to know how the transport of tracers depends on the geographical resolution of the general circulation model. However, this aspect has been scarcely investigated until now. Here, we analyse tracer transport in the ECHAM5 general circulation model using 6 independent idealized tracers with constant lifetimes, which are released in two different altitudes at the surface and in the stratosphere, respectively. Model resolutions from T21L19 to T106L31 were tested by performing multi-annual simulations with prescribed sea surface temperatures and sea ice fields of the 1990s. The impacts of the tracer lifetime were investigated by varying the globally uniform exponential decay time between 0.5 and 50 months. We also tested the influence of using prescribed meteorological fields (ERA40) instead of climatological sea surface temperature and sea ice fields. Meridional transport of surface tracers decreases in the coarse resolution model due to enhanced vertical mixing, with the exception of the advection into the tropical region, which shows an inconsistent trend between the resolutions. Whereas, the meridional transport of tracers released in the stratosphere was enhanced with higher model resolutions, except in the transport from tropical stratosphere to the Southern Hemisphere, which exhibits an increase trend with increasing model resolution. The idealized tracers exhibit a seasonal cycle, which is modulated by the tracer lifetime. In comparison to the run with prescribed sea surface temperature and sea ice fields, the simulation with prescribed meteorological fields did not exhibit significant change in the meridional transport, except in the exchange of stratospheric tracers between both hemispheres, where it causes about 100% increase. The import of the surface tracers into the stratosphere is increased by up to a factor of 2.5, and the export from the stratosphere into the troposphere was increased by up to 60% when prescribed meteorological fields is used. The ERA40 simulation also showed larger interannual variability (up to 24% compared to 12% in the standard simulations). Using our surface tracers released in either the northern or Southern Hemisphere, respectively, we calculate inter-hemispheric transport times between 11 and 17 months, consistent with values reported in the literature. While this study cannot be used to relate differences in model results to specific changes in transport processes, it nevertheless provides some insight into the characteristics of tracer transport in the widely used ECHAM5 general circulation model.

Highlights

  • Transport plays a crucial role in determining the distribution of gas-phase and particulate trace constituents in the atmosphere

  • This study extends the analysis of the ECHAM5 model by testing the sensitivity of the transport of tracers emitted at 6 different locations in the model, in order to answer three major questions: (1) How sensitive is the transport of tracers to model resolution? (2) How does a change in prescribed meteorology and tracer lifetime affect tracer transport? (3) What are the characteristic time scales for inter-hemispheric transport?

  • Transport of the surface tracers is both influenced by the horizontal and vertical resolution of the model, especially at the tropical region, where it monotonically increases with higher number of both resolutions

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Summary

Introduction

Transport plays a crucial role in determining the distribution of gas-phase and particulate trace constituents in the atmosphere. Numerical models are an essential tool for simulating atmospheric transport and distribution of trace species. The ability of a model to simulate the observed distributions of these trace species is largely dependent on its capability to reproduce the transport and mixing of the real atmosphere. Aghedo et al.: Sensitivity of tracer transport in ECHAM5 resolution plays an important role. By comparing the results from different model resolutions, idealized tracers may explain some of the discrepancies observed in the distribution or seasonality of atmospheric trace species in different models These include the analysis of the global characteristics of tracer transport, the discussion of the transport from the source regions into various receptor regions, and the calculation of the interhemispheric transport time in Sect.

The ECHAM5 general circulation model
Experiment description
The influence of model configuration on the global transport characteristics
Meridional transport
Vertical transport
Inter-hemispheric transport time
Findings
Summary and conclusions
Full Text
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