Abstract
Polymers are extensively exploited as active materials in a variety of electronics and energy devices because of their tailorable electrical properties, mechanical flexibility, facile processability, and they are lightweight. The polymer devices integrated with self-healing ability offer enhanced reliability, durability, and sustainability. In this Review, we provide an update on the major advancements in the applications of self-healing polymers in the devices, including energy devices, electronic components, optoelectronics, and dielectrics. The differences in fundamental mechanisms and healing strategies between mechanical fracture and electrical breakdown of polymers are underlined. The key concepts of self-healing polymer devices for repairing mechanical integrity and restoring their functions and device performance in response to mechanical and electrical damage are outlined. The advantages and limitations of the current approaches to self-healing polymer devices are systematically summarized. Challenges and future research opportunities are highlighted.
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