Abstract
In this paper, two comparisons between the two types of rate expressions (i.e. time and surface-oxygen absorption dependence) are provided to answer an important remaining fundamental question from an earlier numerical study by us in 1986. The time-dependent model appears to give a longer time-to-ignition than that predicted by another model type. It is concluded that the two types of chemical rate expressions give inherent differences between their predictions of self-ignition. It is very important to use the conceptually correct model, i.e. the surface-oxygen absorption-dependent rate model, in practical prediction of time-to-ignition.
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