Abstract

The isotope selectivity of computed tomography (CT) imaging based on nuclear resonance fluorescence (NRF) transmission method using a quasi-monochromatic laser Compton scattering (LCS) gamma-ray beam in the MeV region was demonstrated at the Ultra Violet Synchrotron Orbital Radiation-III (UVSOR-III) Synchrotron Radiation Facility (Institute of Molecular Science, National Institute of Natural Science) for two enriched lead isotope rods ( <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">206</sup> Pb and <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">208</sup> Pb) implanted in an aluminum cylinder. Since these two rods show the same gamma-ray attenuation in atomic processes, it is impossible to differentiate between them using a standard Gamma-CT technique based on atomic attenuation of gamma rays. The LCS gamma-ray beam had a maximum energy of 5.528 MeV and an intensity of approximately 5.5 photons/s/eV at the resonance energy (J <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">π</sup> = 1 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">-</sup> at 5.512 MeV in <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">208</sup> Pb). A lead collimator with a hole diameter of 1 mm was used to define the size of the LCS gamma-ray beam at the CT target. The CT image of the <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">208</sup> Pb rod was selectively obtained with a 2-mm pixel size resolution, which was determined by the horizontal step size of the CT stage.

Highlights

  • Science) for two enriched lead isotope rods (206 Pb and 208 Pb) implanted in an aluminum cylinder

  • Takehito Hayakawa and Toshiyuki Shizuma are with the Tokai Quantum Beam Science Center, National Institutes for Quantum and Radiological Science and Technology (QST), Naka 319-1106, Japan (e-mail: hayakawa.takehito@qst.go.jp; shizuma.toshiyuki@qst.go.jp)

  • Masaki Fujimoto is with the National Institute of Natural Science, Institute of Molecular Science, Ultra Violet Synchrotron Orbital Radiation (UVSOR) Synchrotron Radiation Facility, Okazaki 444-8585, Japan (e-mail: fmoto@ims.ac.jp)

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Summary

I NTRODUCTION

ONDESTRUCTIVE assay (NDA) technology, which is used to identify specific isotopes in a substance, Manuscript received March 13, 2020; revised May 29, 2020; accepted. Bertozzi et al [1] proposed the nuclear resonance fluorescence (NRF) process [6] with Bremsstrahlung gamma-ray beams for the measurement of the isotopes of interest. The aim of this study was to demonstrate the isotope selectivity of NRF-CT imaging using two different isotope-enriched lead rods (206 Pb and 208 Pb) Because these two rods exhibit the same gamma-ray attenuation in atomic processes, it is impossible to distinguish the two rods using a standard CT technique based on the atomic attenuation of gamma rays. The energy of the gamma-ray beam was increased to enable excitation at 5.512 MeV, as the NRF cross section was two times larger than that at 5.292 MeV in previous work [16]. An increased number of data points were measured using an LCS beam with a smaller diameter of 1 mm and a scanning step of 2 mm to obtain a CT image with a higher spatial resolution than the previous work [16]

E XPERIMENTAL P ROCEDURE
Findings
R ESULTS AND D ISCUSSION

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