Abstract
The second-order integral equation formalism of Attard, applied recently, with good results, to one-component hard spheres and Lennard-Jones fluids, is applied to some binary mixtures of Lennard-Jones fluids. Comparison with molecular dynamic simulations of the pair correlation functions shows that this method is also quite accurate for mixtures. This is true not only when the Lorentz–Berthelot mixing rules are obeyed but also when there are substantial deviations from these rules.
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