Abstract

Abstract Multiple mechanisms have been proposed to explain secondary ice production (SIP), and SIP has been recognized to play a vital role in forming cloud ice crystals. However, most weather and climate models do not consider SIP in their cloud microphysical schemes. In this study, in addition to the default rime splintering (RS) process, two SIP processes, namely, shattering/fragmentation during freezing of supercooled rain/drizzle drops (DS) and breakup upon ice–ice collisions (BR), were implemented into a two-moment cloud microphysics scheme. Besides, two different parameterization schemes for BR were introduced. A series of sensitivity experiments were performed to investigate how SIP impacts cloud microphysics and cloud phase distributions in warm-based deep convective clouds developed in the central part of Europe. Simulation results revealed that cloud microphysical properties were significantly influenced by the SIP processes. Ice crystal number concentrations (ICNCs) increased up to more than 20 times and surface precipitation was reduced by up to 20% with the consideration of SIP processes. Interestingly, BR was found to dominate SIP, and the BR process rate was larger than the RS and DS process rates by four and three orders of magnitude, respectively. Liquid pixel number fractions inside clouds and at the cloud top decreased when implementing all three SIP processes, but the decrease depended on the BR scheme. Peak values of ice enhancement factors (IEFs) in the simulated deep convective clouds were 102–104 and located at −24°C with the consideration of all three SIP processes, while the temperature dependency of IEF was sensitive to the BR scheme. However, if only RS or RS and DS processes were included, the IEFs were comparable, with peak values of about 6, located at −7°C. Moreover, switching off the cascade effect led to a remarkable reduction in ICNCs and ice crystal mass mixing ratios. Significance Statement The cloud phase is found to have a significant impact on cloud evolution, radiative properties, and precipitation formation. However, the simulation of the cloud phase is a big challenge for cloud research because multiple processes are not well described or missing in numerical models. In this study, we implemented two secondary ice production (SIP) processes, namely, shattering/fragmentation during the freezing of supercooled rain/drizzle drops and breakup upon ice–ice collisions, which are missing in most numerical models. Sensitivity experiments were conducted to investigate how SIP impacts cloud microphysics and cloud phase in deep convective clouds. We found that SIP significantly impacts in-cloud and cloud-top phase distribution. We also identified that the collisional breakup of ice particles is the dominant SIP process in the simulated deep convective clouds.

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