Abstract
Three new orthopalladated chromophores based on push–pull π conjugated ligands have been prepared and characterized. The second order molecular NLO activity has been determined by EFISH measurements giving μgβ values up to 610×10−48 esu at an incident laser wavelength of 1.907 μm. The X-ray structures of two different polymorphs of one chromophore are also reported and polymorphism is discussed in terms of conformational changes.
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